Usually, your subscribers can subscribe or unsubscribe by themselves. However, it is possible to unsubscribe one or more contacts manually.
To unsubscribe subscribers from one or more contact lists:
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Browse to the main "Contacts" menu.
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Click on the contact list in wich you want to remove one or more subscriber.
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Browse through the secondary menu "Remove Subscribers" on the right.
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Enter each email address you want to remove on a separate line.
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Click on the "Unsubscribe" button.
Unsubscribing from several contact lists at the same time:
If you have more than one contact list and you want to remove a subscriber thru all your lists, make sure you select the option "Unsubscribe these email addresses from all my contact lists".